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The nanoscale interface for organic electronics refers to the critical contact region, precisely engineered at the atomic or molecular level, between different materials within devices utilizing organic compounds. This ultrathin boundary plays a pivotal role in dictating charge transport, injection efficiency, and overall device performance, stability, and lifetime in applications such as organic light-emitting diodes (OLEDs), organic solar cells, and flexible electronic components, making its control essential for advancing next-generation technologies.